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Cu3Sn was recently predicted to host topological Dirac fermions, but relatedresearch is still in its infancy. The growth of large and high-quality Cu3Snsingle crystals is, therefore, highly desired to investigate the possibletopological properties. In this work, we report the single crystal growth ofCu3Sn by Czochralski (CZ) method. Crystal structure, chemical composition, andtransport properties of Cu3Sn single crystals were analyzed to verify thecrystal quality. Notably, compared to the mm-sized crystals from a moltenSn-flux, the cm-sized crystals obtained by the CZ method are free fromcontamination from flux materials, paving the way for the follow-up works.

Preparation of large Cu3Sn single crystal by Czochralski method