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An ultra-thin FeO(111) film grown on Pt(111) is found to exhibit a much higher rate of CO oxidation at stoichiometric CO:O2 ratios than the clean Pt(111) surface. This unexpected result is rationalized on the basis of reaction induced dewetting of the oxide film, ultimately resulting in highly dispersed FeO x  nanoparticles on Pt(111). The effect may have a strong impact on the catalytic properties of the noble metal particles encapsulated by the reducible oxide support as a result of strong metal-support interaction.

When an Encapsulating Oxide Layer Promotes Reaction on Noble Metals: Dewetting and In situ Formation of an “Inverted” FeO x /Pt Catalyst