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Palladium-iron alloys produced by high-dose implantation of iron ions intoepitaxial palladium films were investigated with the ferromagnetic resonance(FMR) and vibrating sample magnetometry (VSM) techniques. The samples revealdistinct multiple FMR responses depending on the dose of iron ion implantation.The post-implantation annealing at 770 K does not bring the implanted films toa homogeneous solid solution state, as might be expected from the Pd-Fe phasediagram. On the contrary, the system approaches a stable state composed ofseveral magnetic phases. FMR spectra exhibit an angular behavior specific for astack of interacting magnetic layers. This observation, correlated with themagnetometry data, indicates that the palladium-iron binary alloy has apreviously unknown tendency towards spinodal decomposition into isostructuralphases with well-defined iron concentrations and, accordingly, with differenttemperatures of ferromagnetic ordering and saturation magnetizations.

Manifestations of Spinodal Decomposition into Dilute Pd$_{1-x}$Fe$_{x}$ "Phases" in Iron-Implanted Palladium Films: FMR Study