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Inspired by the path followed by Matthias Ballauff over the past 20 years,the development of thermosensitive core-shell microgel structures is reviewed.Different chemical approaches, from hard nanoparticle cores to doublestimuli-responsive microgels have been devised and successfully implemented bymany different groups. Some of the rich variety of these systems is presented,as well as some recent progress in structural analysis of such microstructuresby small-angle scattering of neutrons or X-rays, including modeling approaches.In the last part, again following early work by the group of Matthias Ballauff,applications with particular emphasis on incorporation of catalyticnanoparticles inside core-shell structures -- stabilizing the nanoparticles andgranting external control over activity -- will be discussed, as well ascore-shell microgels at interfaces.

Recent advances in stimuli-responsive core-shell microgel particles: synthesis, characterisation, and applications