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A series of bicationic monochromophoric hemicyanine dyes based on benzothiazolestyrylium residues were synthesized. The dyeing photoinitiating systems consisting of N -[3-(4-methylpyridino)propyl]-2-( p -substituted styryl)benzothiazolium dihalides as chromophores and n -butyltriphenylborate anion as electron donor were also prepared to achieve an efficient photoinitiators for free-radical polymerization in a visible-light region. The relative photoinitiating efficiencies of novel photoinitiators of acrylate monomers polymerization were evaluated.

Visible light-induced polymerization initiated by borate salts of bicationic monochromophoric benzothiazolestyrylium dyes