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The author's work on the reactions of Cp 2 Mo 2 Co 2 S 3 (CO) 4 (1) and Cp 2 Mo 2 Co 2 S 4 (CO) 2 (2) with organosulfur compounds is reviewed. Reaction pathways that lead to C S bond scission are proposed, and the relexance of these results to HDS reactions mer commercial “CoMoS” catalysts is discussed

Electron-deficient molybdenum/cobalt/sulfido clusters: Chemistry related to hydrodesulfurization (HDS) catalysis