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The following temperature-dependent rate coefficients (k/cm3 molecule-1 s-1) of the reactions of hydroxyl radicals with aliphatic ethers have been determined over the temperature range 247–373 K by a competitive flow technique: diethyl ether,kOH=5.2×10-12 exp[(262±150)/T]; methyln-butyl ether,kOH=5.4×10-12 exp[(309±150)/T]; ethyln-butyl ether,kOH=7.3×10-12 exp[(335±150)/T]; di-n-butyl ether,kOH=5.5×10-12 exp[(502±150)/T] and di-n-pentyl ether,kOH=8.5×10-12 exp[(417±150)/T]. The data have been measured relative to the rate coefficientk(OH + 2,3-dimethylbutane)=6.2×10-12 cm3 molecule-1 s-1 independent of temperature.

journal of atmospheric chemistry

Further studies of the temperature dependence of the rate coefficients for the reactions of OH with a series of ethers under simulated atmospheric conditions