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Summary  Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the “BBO family,” including BBO, CLBO, KABO, KBBF, RBBF, CBBF, BABF, BiBO, LBO, CBO, LRB4, LCB, YCOB, and GdCOB. They satisfy three kinds of group‐velocity matching condition from near‐infrared to telecom wavelengths. Furthermore, heralded single photons can be generated with a purity as high as 0.98, which is achieved without any narrow filtering. The indistinguishability of photons from independent sources is examined by the Hong‐Ou‐Mandel interference, which results in a visibility of 98% also without any further filtering, that is, photons from different heralded single‐photon sources are highly indistinguishable. Our study may provide single‐photon sources with good performance for quantum information processing at near‐infrared and telecom wavelengths.

Spectrally uncorrelated biphotons generated from “the family of BBO crystal”