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Autoignition delay times, ?, of methyl crotonate, methyl acrylate, ethylbutanoate, ethyl crotonate, and ethyl acrylate were studied in shock tubeexperiments. A series of mixtures diluted with argon, of varying fuel/oxygenequivalence ratios (?=0.25, 0.4, 1.0, and 2.0), were measured behind reflectedshock waves over the temperature range of 1280-1930 K, pressure range of 7-9.65atm, during which the logarithm of ? varies linearly as a function of theinverse temperature for all equivalence ratios. The ignition delay timedecreases as temperature rises. The dependence of ? on temperature, andreactant concentrations is given in an empirical correlation. The resultsprovide a database for the validation of small saturated and unsaturated esterskinetic mechanisms at elevated temperatures and pressure combustion.

Experimental Autoignition of C4-C6 Saturated and Unsaturated Methyl and Ethyl Esters