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Using density functional theory, we have investigated the electronic andmagnetic properties of finite-size as well as infinitely periodicorganometallic vanadium-borazine systems for their possible applications inspintronics devices. From our calculations, we find the finite-sizevanadium-borazine systems to be structurally more stable in comparison to theirisoelectronic benzene counterparts. All the finite-size vanadium-borazinesystems are found to be ferromagnetically stabilized, with the infiniteone-dimensional wire exhibiting robust half-metallic behaviour. The finite-sizeclusters are also found to exhibit efficient spin filter properties whencoupled to graphene electrodes.

Organometallic Vanadium-Borazine Systems: Efficient One- Dimensional Half-Metallic Spin Filters