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We have studied the magneto-optical Kerr effect and optical reflectance ofperpendicular magnetized Co/Pt films on self-assembly two-dimensionalpolystyrene spheres. It is shown that the magneto-optical and the reflectancespectra are correlated to each other. Calculations have shown that themagneto-optical Kerr rotation and the Kerr ellipticity spectra are governed bythe resonant coupling of light to the excitations of surface plasmon polaritonsand modified by the sphere diameters. These effects lead to the possibility ofdeveloping new magnetoplasmonic nanosensors.

Anomalous magneto-optical Kerr effect in perpendicularly magnetized Co/Pt films on two-dimensional colloidal crystals