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The tetragonal layered compounds TbTiGe and ErTiGe orderantiferromagnetically at 276 K and 39 K, respectively. Partial substitution ofMo for Ti in these two compounds modifies the magnetic interactions giving riseto a ferromagnetic ground state which results in an enhanced magnetocaloriceffect. The magnetic entropy change in ErTi0.85Mo0.15Ge for a magnetic fieldchange of 5 T is ~10.5 J/kg/K against ~0.8 J/kg/K for ErTiGe in the vicinity ofthe magnetic transition. Thus, magnetocaloric properties of such layeredmaterials may be tunable by suitable chemical substitutions.

Tuning the Competing magnetic interactions in RTiGe (R = Tb, Er) Compounds and tailoring the Magnetocaloric effect