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The structure, electronic, and magnetic properties of the Mo-doped perovskiteLa0.7Ca0.3Mn1-xMoxO3 (x < 0.1) have been studied. A significant increase inresistivity and lattice parameters were observed with Mo doping. A marginaldecrease in the Curie temperature Tc and the associated metal-insulatortransition Tp were observed. Magnetization data reveal that long-rangeferromagnetic ordering persists in all samples studied and the saturationmoment decreases linearly as x increases. Enhancement in magnetoresistance atnear Tc in the Mo-doped compounds with an optimum doping value x = 0.05 wasobserved. The overall experimental results can be explained by considering theinduced Mn2+ ions with Mo6+ in the Mo-doped systems, with the strong FMcoupling between Mn4+/2+- O - Mn3+.

Effect of Mo doping for the Mn site in the ferromagnetic manganite La0.7Ca0.3MnO3