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We propose a method for enantio-detection of chiral molecules based on acavity-molecule system, where the left- and right-handed molecules are coupledwith a cavity and two classical light fields to form cyclic three-level models.Via the cavity-assisted three-photon processes based on the cyclic three-levelmodel, photons are generated continuously in the cavity even in the absence ofexternal driving to the cavity. However, the photonic fields generated from thethree-photon processes of left- and right-handed molecules differ with thephase difference {\pi} according to the inherent properties of electric-dipoletransition moments of enantiomers. This provides a potential way to detect theenantiomeric excess of chiral mixture by monitoring the output field of thecavity.

Enantio-detection via cavity-assisted three-photon processes