Multielectron effects in the photoelectron momentum distribution of noble-gas atoms driven by visible-to-infrared-frequency laser pulses: A time-dependent density-functional-theory approach
Author(s) -
Mitsuko Murakami,
G. P. Zhang,
ShihI Chu
Publication year - 2017
Publication title -
physical review. a/physical review, a
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.391
H-Index - 283
eISSN - 2469-9934
pISSN - 2469-9926
DOI - 10.1103/physreva.95.053419
Subject(s) - neon , time dependent density functional theory , atomic physics , density functional theory , ionization , physics , electron , laser , argon , helium atom , atom (system on chip) , noble gas , helium , excited state , quantum mechanics , ion , embedded system , computer science
We present the photoelectron momentum distributions (PMDs) of helium, neon, and argon atoms driven by a linearly polarized, visible (527-nm) or near-infrared (800-nm) laser pulse (20 optical cycles in duration) based on the time-dependent density-functional theory (TDDFT) under the local-density approximation with a self-interaction correction. A set of time-dependent Kohn-Sham equations for all electrons in an atom is numerically solved using the generalized pseudospectral method. An effect of the electron-electron interaction driven by a visible laser field is not recognizable in the helium and neon PMDs except for a reduction of the overall photoelectron yield, but there is a clear difference between the PMDs of an argon atom calculated with the frozen-core approximation and TDDFT, indicating an interference of its M-shell wave functions during the ionization. Furthermore, we find that the PMDs of degenerate p states are well separated in intensity when driven by a near-infrared laser field, so that the single-active-electron approximation can be adopted safely.
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