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Wavelength‐Tunable Microlasers Based on the Encapsulation of Organic Dye in Metal–Organic Frameworks
Author(s) -
Wei Yanhui,
Dong Haiyun,
Wei Cong,
Zhang Wei,
Yan Yongli,
Zhao Yong Sheng
Publication year - 2016
Publication title -
advanced materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 10.707
H-Index - 527
eISSN - 1521-4095
pISSN - 0935-9648
DOI - 10.1002/adma.201601844
Subject(s) - materials science , lasing threshold , metal organic framework , broadband , optoelectronics , encapsulation (networking) , wavelength , organic dye , nanotechnology , computer science , telecommunications , chemical engineering , chemistry , organic chemistry , adsorption , engineering , computer network
A wavelength‐tunable microlaser is realized based on the controlled intramolecular charge transfer (ICT) process in dye‐encapsulated metal–organic framework (MOF) material. The confinement effect of the MOFs is beneficial for low‐threshold lasing. By effectively controlling the polarity of the MOF pores, the population distribution between the locally excited and ICT states is continuously modulated, thus achieving broadband tunable MOF‐based microlasers.
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