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Ionic liquids are room-temperature molten salts, composed of organic mostly of organic ions that may undergo almost unlimited structural variation. We approach the new aspects of ionic liquids in applications where the semiconductor nanoparticles used as sensitizers of solar cells. We studied the effects of ionic liquids as capping ligand and/or solvent, on the morphology and phase of the CdSe/ZnS nanoparticles. Colloidal CdSe/ZnS nanoparticles were synthesized using a series of imidazolium ionic liquids; 1-R-3-methylimidazolium bis(trifluoromethylsulfo- nyl)imide ((RMIM)(TFSI)), where R = ethyl ((EMIM)), butyl ((BMIM)), hexyl ((HMIM)), octyl ((OMIM)). The average size of nanoparticles was 8~9 nm, and both zinc-blende and wurtzite phase was produced. We also synthesized the nanoparticles using a mixture of trihexyltetrade- cylphosphonium bis(trifluoromethylsulfonyl)imide ((P6,6,6,14)(TFSI)) and octadecene (ODE). The CdSe/ZnS nanoparticles have a smaller size (5.5 nm) than that synthesized using imidazolium, and with a controlled phase from zinc-blende to wurtzite by increasing the volume ratio of

Phase-and Size-Controlled Synthesis of CdSe/ZnS Nanoparticles Using Ionic Liquid