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Boron trifluoride lithium methacrylate (LiMA)-based gel polymer electrolytes (GPEs) were synthesized with various LiMA concentration to elucidate the effect on ionic conductivity and electrochemical stability by a AC impedance and linear sweep voltammetry (LSV). As a result, the highest ionic conductivity reached at was obtained for 4 wt% of LiMA. Furthermore, high electrochemical stability up to 4.3 V of the LiMA-based GPE was observed in LSV measurement since the counter anion was immobilized in this self-doped system. On the other hand, it was assumed that there was a rapid decomposition of electrolytes on a lithium metal electrode which results in a high solid electrolyte interface (SEI) resistance. However, a high stability toward graphite or lithium cobalt oxide (LCO) electrode thereby a low SEI resistance was observed from the AC impedance measurement as a function of storage time at . Consequently, the high ionic conductivity, good electrochemical stability and the good interfacial compatibility with graphite and LCO were achieved in LiMA-based GPE.

Effect of Lithium Ion Concentration on Electrochemical Properties of BF3LiMA-based Self-doping Gel Polymer Electrolytes

Effect of Lithium Ion Concentration on Electrochemical Properties of BF₃LiMA-based Self-doping Gel Polymer Electrolytes