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The PartMC-MOSAIC particle-resolved aerosol model was previously developed to\udpredict the aerosol mixing state as it evolves in the atmosphere. However,\udthe modeling framework was limited to a zero-dimensional box model approach\udwithout resolving spatial gradients in aerosol concentrations. This paper\udpresents the development of stochastic particle methods to simulate turbulent\uddiffusion and dry deposition of aerosol particles in a vertical column within\udthe planetary boundary layer. The new model, WRF-PartMC-MOSAIC-SCM, resolves\udthe vertical distribution of aerosol mixing state. We verified the new\udalgorithms with analytical solutions for idealized test cases and illustrate\udthe capabilities with results from a 2-day urban scenario that shows the\udevolution of black carbon mixing state in a vertical column

A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0