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We used chemical ionization mass spectrometry with a volatilizationflow tube inlet (Aerosol-CIMS) to characterize secondary organicmaterial formed by methylglyoxal with ammonium sulfate in aqueousaerosol mimics. Bulk reaction mixtures were diluted and atomized toform submicron aerosol particles. Organics were detected usingAerosol-CIMS in positive and negative ion mode using I− andH3O+·(H2O)n as reagent ions. The results areconsistent with aldol condensation products, carbon-nitrogen species,sulfur-containing compounds, and oligomeric species up to759 amu. These results support previous observations by us andothers that ammonium sulfate plays a critical role in the SOAformation chemistry of dicarbonyl compounds

Secondary organic material formed by methylglyoxal in aqueous aerosol mimics