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Silica-supported P2O5 (P2O5/SiO2) was used as an efficient, green and cheap catalytic system for the synthesis of N-sulfonyl imines via condensation of sulfonamides with several aldehydes under solvent-free conditions. The reactions proceeded rapidly at 110 °C and the desired products were obtained in high to excellent yields.

P2O5/SiO2 an efficient, green and heterogeneous catalytic system for the solvent-free synthesis of N-sulfonyl imines