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A novel approach for the synthesis of 2,3-dihydro-1H-1,5-benzodiazepines from o-phenylenediamines and structurally divergent ketones is described using zinc montmorillonite as catalyst at room temperature. The catalyst can be reused for at least three cycles with consistent activity.

Zinc montmorillonite as a reusable heterogeneous catalyst for the synthesis of 2,3-dihydro-1H-1,5-benzodiazepine derivatives