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The intramolecular aldol condensation of 3-oxocyclohexaneacetaldehydes leading to C(6) epimeric mixtures of 6-hydroxybicyclo[2.2.2]octan-2-ones is reviewed. Both steps, the preparation of the 3-oxocyclohexaneacetaldehyde and its cyclization were examined, as well as applications to the synthesis of natural products.

The intramolecular aldol condensation of 3-oxocyclohexaneacetaldehydes: a useful tool in the synthesis of natural products