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Under flash vacuum pyrolysis (FVP) conditions a number of competitive routes are available for the thermal cleavage of 1,5-diazapentadienes (vinamidines) and their aza-analogues. First, the 6π ‘electrocyclisation with elimination’ route to quinolines 2 and related compounds (Scheme 1), pioneered by Jutz and co-workers in condensed-phase, is observed exclusively in the gas-phase only for 1,5-diarylvinamidines 1.

Thermolysis of polyazapentadienes. Part 12.1 The 1,1-dialkyl-5-aryl-1,3,5-triazapentadiene problem