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A series of 9-amino-10-arylanthracenes was easily prepared from bromobenzene and arylacetonitriles via benzyne and α-lithiated 2-arylmethylbenzonitrile intermediates. In addition, several mono-, di-, tri-, and tetra-peri-substituted derivatives of 10-aryl-9- aminoanthracenes and 9,10-dihydroanthracen-9-imines were obtained from the reaction of the respective bromoarenes as precursors of in situ generated benzyne, 3-methoxy-, 6-methoxy-3- methyl-, and 3-,6-dimethoxybenzyne with preformed α-lithiated 2-arylmethyl-benzonitriles.

Facile one-pot synthesis of 10-aryl derivatives of 9-aminoanthracenes and 9,10-dihydroanthracen-9-imines