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Photoelectrochemical (PEC) water splitting is a promising strategy to improve the efficiency of oxygen evolution reactions (OERs). However, the efficient adsorption of visible light as well as long-term stability of light-harvesting electrocatalysis is the crucial issue in PEC cells. Metal-organic framework (MOF)-derived bimetallic electrocatalysis with its superior performance has wide application prospects in OER and PEC applications. Herein, we have fabricated a nickel and iron bimetallic organic framework (FeNi-MOF) deposited on top of anodized TiO 2 nanotube arrays (TNTA) for PEC and OER applications. The FeNi-MOF/TNTA was incorporated through the electrochemical deposition of Ni 2+ and Fe 3+ onto the surface of TNTA and then connected with organic ligands by the hydrothermal transformation. Therefore, FeNi-MOF/TNTA demonstrates abundant photoelectrocatalytic active sites that can enhance the photocurrent up to 1.91 mA/cm 2 under 100 mW/cm 2 and a negligible loss in activity after 180 min of photoreaction. The FeNi-MOF-doped photoanode shows predominant photoelectrochemical performance due to the boosted excellent light-harvesting ability, rapid photoresponse, and stimulated interfacial energy of charge separation under the UV-visible light irradiation conditions. The results of this study give deep insight into MOF-derived bimetallic nanomaterial synthesis for photoelectrochemical OER and provide guidance on future electrocatalysis design.

nanomaterials

Fe/Ni Bimetallic Organic Framework Deposited on TiO2 Nanotube Array for Enhancing Higher and Stable Photoelectrochemical Activity of Oxygen Evaluation Reaction