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Relative partial molar Gibbs energies of the Mg component substituted into the Zn site, ΔG Mg Mg on Zn site , in the intermediate phases of Mg 0.48 Zn 0.52 and Mg 0.4 Zn 0.6 in the Mg-Zn binary system were directly evaluated, assuming that change in the chemical potential of magnesium, Δμ Mg , as a function of the composition in a narrow solubility limit is caused by anti-site substitution of Mg atoms at the Zn site. At 298 K, the AG Mg Mg on Zn site values of Mg 0.4 Zn 0.6 and Mg 0 . 48 Zn 0.52 were found to be 1.254 and 0.163 MJ·mol ―1 , respectively, consistent with about the same order of internal energy of the Fe components substituted into the Pt site, ΔU Fe Fe on Pt site , in the ordered phase of Ll 0 -Fe 1―x Pt x calculated by theoretical calculation (= 0.101 MJ·mol ―1 ). When the symmetric atomic configuration at the stoichiometric composition was violated by anti-site substitution, the relative partial molar thermodynamic value of lattice defect was found to be very large.

Relative Partial Molar Gibbs Energy of Magnesium Component Substituted into Zinc Site in the Mg-Zn Binary Compounds