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Three-dimensional potential energy functions have been generated  ab initio  for the  X  2 Π electronic ground state of CCS −  and used in variational Renner–Teller calculations including electron spin. Rovibronic levels ( J = P ) for  J ≤5/2 are given for energies up to 4000cm −1 . The pattern of the levels is compared with that of CCO − . In the case of CCS −  the quartic force fields, equilibrium geometry, electric dipole moment, the electronic affinity and the Franck–Condon factors for the  X  2 Π(CCS − ) →  X  3 Σ −  (CCS) photodetachment spectrum are calculated.

Rovibronic States in the X 2 Π State of the CCS − Anion