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The recently observed linear dependence of the lifetime of excited hydrated electrons upon the inverse of the cluster size is explained in terms of a nonadiabatic long range coupling mechanism. It is due to dipolar interactions between the  p → s  transition and the excitation of the infrared active modes of the solvent water molecules.

Long Range Nonadiabatic Couplings and the Cluster-Size Dependence of the Lifetime of Excited Hydrated Electrons