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The thermodynamic dissociation constants for isoelectric reaction of the type LH +   ↔ L + H +  (where L = 2,2´-bipyridine or 1,10-phenanthroline) have been determined pH-metrically at 298°K in aqueous binary mixtures of tetrahydrofuran (0-90 wt% of organic co-solvent). The pK-values have been found to decrease continuously. The data have been utilized to calculate the Gibbs energies of transfer of H + -ion from water to tetrahydrofuran-water mixtures. The results have been explained in terms of ion-solvent interactions, structural variations and basicity of aquo-organic mixtures.

Gibbs Energies of Transfer of Hydrogen Ion from Water to Tetrahydrofuran + Water Mixtures and Basicity and Structuredness of Aquo-ethers