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Fluorescence spectroscopy was used to study the Ca 2+ /UO 2  2+ /CO 3  2-   solution system at different ionic strengths. Fluorescent titrations confirmed formation of Ca 2 UO 2 (CO 3 ) 3  complex for which the values of log β 213  were measured at 0.1, 0.3, 0.7, 1.0 and 3.0 m (NaClO 4 ) at pcH = 8.1. Specific Interaction Theory (SIT) was used to correlate the log β 213  values as a function of ionic strength. The value obtained for log β 0  213  (I = 0) was 29.8 ± 0.7, indicating that Ca 2 UO 2 (CO 3 ) 3  was the predominant specie at the pH 8 in calcium rich, oxic waters.

Mixed Ca 2+ /UO 2 2+ /CO 3 2- complex formation at different ionic strengths