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The crystalline structure and quality of ZnSnAs 2 :Mn films grown by molecular beam epitaxy (MBE) on InP substrates are two of the most important issues in preparing spintronic structures such as magnetic quantum wells and spin-based transistors. We conducted high-resolution X-ray diffraction (XRD) measurements to clarify the crystalline structure of ZnSnAs 2 :Mn thin films. The XRD measurements reveal with very high accuracy that the samples have a sphalerite structure with high epitaxial quality. These results, within the limits of measurement accuracy support the previous assumption that ZnSnAs 2 :Mn thin films are coherently clustered ferromagnetic semiconductors without breaking the continuity of the sphalerite structure, leading to ferromagnetism with a high Curie temperature close to that of zincblende MnAs.

zeitschrift für physikalische chemie

Crystalline Quality and Structure of MBE-Grown Ferromagnetic Semiconductor ZnSnAs 2 :Mn Thin Films Revealed by High-Resolution X-ray Diffraction Measurements