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A new complex [Pr 3 NH] +  [Mn(dca) 3 ] −  · H 2 O (dicyanamide = dca − ) was synthesized, in which the Mn 2+  cations are bridged by end-to-end dca anions to form three-dimensional [Mn(dca) 3 ]  n  n   −  networks and tripropylammonium cations reside in the cavities of these networks. The complex has been characterized by single-crystal X-ray diffraction, infrared spectroscopy, elemental analysis, and magnetic measurements. Magnetic susceptibility data indicate ferromagnetic interactions among the Mn II  ions.

Ferromagnetic interactions in a dicyanamide-bridged multinuclear metal-organic framework [Pr 3 NH] + [Mn(dca) 3 ] − ·H 2 O