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The compound H 5 C 6 (H)Ge[C(GaCMe 3 )=C(H)CMe 3 ] 2 (μ-H) 3 [Ga(CMe 3 ) 2 ],  2 , was isolated in trace quantities from the reaction of Et 2 N–Ge(C≡C–CMe 3 ) 3  with excess H–Ga(CMe 3 ) 2 . Compound  2  has a unique molecular structure with a Ga 3 H 3  heterocycle of which one Ga–H–Ga group is bridged by a dialkenylgermanium unit. The molecular structure of a second compound ( 3 ) is reported, which may be described as a  spiro -germane and has AlNGeC and AlC 2 Ge heterocycles. The rings are formed by intramolecular Al–N and Al–C interactions.

Hydrometallation of amino-dialkynylgermanes – a gallium hydride oligomer and intramolecular Lewis acid-base interactions