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The dicarbene platinum complexes of the type [Pt(L) 2 ]Br 2  [5]Br 2  - [8]Br 2  (L = N-alkyl-N´- picolylbenzimidazolin-2-ylidene) have been prepared by two different methods. The in situ deprotonation of picoline-functionalized benzimidazolium salts 1 - 4 with platinum acetylacetonate gave the platinum complexes [5]Br 2  - [8]Br 2  in good yields. Complex [8]Br 2  has also been obtained by a ligand transfer reaction from the silver dicarbene complex [9][AgBr 2 ]. Attempts to cystallize [8]Br 2  obtained from the carbene transfer reaction led to the isolation of the previously undetected monocarbene complex [Pt(Cl) 2 L] (10) which contains only one picoline-functionalized carbene ligand coordinating in a chelating fashion to the metal center

Platinum Complexes with Picoline-functionalized Benzimidazolin-2-ylidene Ligands