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1,3-Diisopropyl-4,5-dimethylimidazolium acetylacetonate (2) is obtained from 2,3-dihydro-1,3-diisopropyl-4,5-dimethylimidazol- 2-ylidene (1) and acetylacetone. Its crystal structure reveals the presence of ion pairs linked by C-H ··· O hydrogen bonds. In 2, the acetylacetonate ion adopts the structure of its E/Z-isomer (C).

The Acetylacetonate Ion as its E/Z-Isomer in 1,3-Diisopropyl-4,5- dimethylimidazolium Acetylacetonate