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The EPR g factors of Cr 3+  in NaCrS 2  and NaCrSe 2  crystals are calculated from the high-order perturbation formulas based on the one-spin-orbit (SO)-coupling-parameter (i. e., the SO-couplingparameter of the central 3d n  ion) as well as the two-SO-coupling-parameter (i. e., the SO-couplingparameter of the 3d n  ion and that of ligands) models for 3d n  ions in cubic octahedral sites. The calculated results (in particular for NaCrSe 2 ) based on the two-SO-coupling-parameter model are closer to the observed values than those based on the one-SO-coupling-parameter model, suggesting that for calculations of the g factor of 3d n  ions in covalent crystals the two-SO-coupling-parameter model is preferable to the one-SO-coupling-parameter model. The reasonableness of the calculated results from the two-SO-coupling-parameter model is discussed.

Investigations Of The Epr G Factors Of Nacrs 2 And Nacrse 2