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With the help of a microwave Fourier transform spectrometer in the range from 18 GHz to 26 GHz, the coefficients ß for the linear pressure depedence of collisional dephasing rates 1/T 2  have been determined by the transient emission technique for fourteen pure rotational transitions of SO 2  with 5 ≦ J' ≦ 66 in the ground vibrational state, twelve transitions with 8 ≦ J' ≦ 62 in the first excited bending vibrational state, and twelve transitions of methanol with 2 ≦ J' ≦ 11, where J' is the rotational quantum number of the upper level of a transition. The T 2 -parameter ß for the transition J(K - , K + ) - 49(4, 46 ) - 48(5, 43) of SO 2  in the ground state shows an anomalous behaviour, whereas the values for all other transitions show a J-dependence in accordance with previous results. No significant variation of T 2 -parameters with J has been found for the rotational transitions of CH 3 OH.

J-Dependence of T 2 -Parameters for Rotational Transitions of SO 2 and CH 3 OH in K-Band