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A newly designed millimeter-wave spectrometer has been employed for precise measurements of the millimeter-wave rotational spectrum of HCNO. Absorptions in several excited vibrational states as well as the ground state could be measured. The present paper presents the observed frequen­ cies and molecular constants obtained for the ground state and the first excited state of v 4  and of v 5 , the vibrational bending modes

Centrifugal Distortion Parameters of Fulminic Acid, HCNO, from the Millimeter-Wave Rotational Spectra