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Self-assembled monolayers (SAMs) of alkanethiols on gold have been one of the most well studied systems. The SAM with a photoactive group and an electron relay group formed on a metal electrode in a solution containing an electron acceptor and/or donor should be a good candidate for a stable, efficient photoconversion device where up-hill photoinduced electron transfer, i.e., photocurrent generation, takes place. We have achieved a control of a direction of photoinduced electron transfer and a very efficient photocurrent generation at the gold electrodes modified with the SAMs of porphyrin-quinone-thiol and porphyrin-ferrocene-thiol linked molecules.

hyōmen kagaku/hyoumen kagaku

Frontiers of Photo-catalysis and Photo-reaction at Solid Surfaces. Visible-Light-Induced Electron Transfer at Electrodes Modified with Self-Assembled Monolayers.