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Octave-spanning, 12.5 fs, (1.9 cycle) pulses with 115 {\mu}J energy in theshort-wavelength mid-infrared spectral range (1-2.5 {\mu}m) have been generatedvia phase-mismatched cascaded nonlinear frequency conversion using organic DASTcrystal. Such ultra-fast cascading effect is ensured by the interaction of apump pulse with the exceptionally large effective nonlinearity of the DASTcrystal and experiencing non-resonant, strongly phase mismatched, Kerr-likenegative nonlinearity.

Intense sub-2 cycle infrared pulse generation via phase mismatched cascaded nonlinear interaction in DAST crystal