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Many nonlinear optical scenarios, including the typical high-order harmonic radiation, can be initiated in crystals exposed to ultrashort strong lasers. According to the recent theoretical calculation, the high-order harmonic radiation can be modulated by exerting the strain on a monolayer aluminum nitride. Since the high-order harmonic spectra carry the structural information of the target, inversely, the radiated spectra can be used to extract the microstructure of the target and even the ultrafast electron dynamics.

From strain engineering of material to photon radiation: a new perspective for investigating crystal microstructure andelectronic structure