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Temperature dependence of the b2(0) spin-hamiltonian parameter for Gd3+ in RbCdF3 single crystals is described. The dependence is interpreted in terms of the 4f7 electrons coupling to the whole phonon spectrum of the crystal. The presented data give also an insight into the dynamics of charge compensators causing a tetragonal distortion of the crystal field.

Spin-Phonon Contributions to the b02Parameter for Gd3+in RbCdF3Single Crystals

Spin-Phonon Contributions to the b⁰₂Parameter for Gd³⁺in RbCdF₃Single Crystals