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In this paper we introduce a new model describing the coupling of 2E and 4T2 states of octahedrally coordinated Cr3+ ion, which includes spin-orbit and electron-lattice interactions and takes into account the electronic structure of both states. The model is used to calculate doublet lifetime. We have applied this model to the series of Cr3+ doped garnets characterized by the varying crystal field parameter 10 Dq and O(h) symmetry of the Cr site and to the kyanite (Al2O3:SiO2), which is the case of different Cr3+ sites in one material, characterized by the relatively large component of the low symmetry crystal field. The agreement with experiment is reasonable.

Spin-Orbit Coupling in Cr3+Ion in Solid State Materials

Spin-Orbit Coupling in Cr³⁺Ion in Solid State Materials