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A general discussion of the simulation procedure of the full susceptibility tensor and isothermal magnetization pseudovector for compounds comprising weakly-interacting magnetic centers is presented. A single-crystal-sample as well as a powder-sample case are considered. The procedure is used to obtain explicit expressions for the full susceptibility tensor for spins S = 1, 3/2, 2, and 5/2 for non-vanishing rhombic local anisotropy and any form of spectroscopic tensor. PACS: 75.10.Dg, 75.10.Jm, 75.30.Gw, 75.50.Xx

Full Susceptibility Tensor for Localized Spin Models with S = 1, 3/2, 2, 5/2 and with Rhombic Anisotropy