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Molecular dynamics (torsional frequencies) in several chlorine compounds were evaluated on the basis of X-ray thermal parameter data and nuclear quadrupole resonance data using Bayer's and Brown's approximation. It was found that the values obtained in both cases are in good agreement. The above approach is a good illustration of the supplementary nature of the data from X-ray studies in relation to nuclear quadrupole resonance studies of compounds in solid state.

Molecular Dynamics in Chlorine Compounds Using X-Ray Thermal Parameters and Nuclear Quadrupole Resonance Data