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The resonance enhanced multiphoton ionization method has been applied to the study of NO-Ar van der Waals complex in the nsσ (n = 3,4) Rydberg states. We have assigned the intermolecular vibrations appearing in the Ã—   X  ˜    excitation spectrum of the complex. The bending structure appeared only with the excitation of the stretching mode in the Ã state, which was interpreted by intermolecular forces. The    E  ˜   -Ã excitation spectra were independent of the initial intermolecular level in the Ã state and the dissociation threshold to NO(E 2∑  +    ) + Ar was determined to be 60950 cm -1 . The s–d mixing in the 4sσ orbital would make the intermolecular vibrational structure in the    E  ˜   —Ãspectra complex.

Intermolecular Vibrations of the Complex of NO in the nsσ Rydberg States and Ar