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Selective enhancement of coherent optical phonons in Bi-Sb mixed crystals hasbeen performed using terahertz (THz) rate pulse trains generated by spatialphase modulation of femtosecond pulse with a liquid-crystal spatial lightmodulator. The profile of the shaped pulse train has a flat-toped shape. TheBi-Bi, Bi-Sb, and Sb-Sb vibrations can be enhanced and canceled selectively forpulse trains with a suitable repetition rate.

Selective enhancement of coherent optical phonons using THz-rate pulse train