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In the title molecular salt, C 20 H 19 N 2 S + ·I − , prepared by the reaction of 1,3-diphenylthiourea and benzyl iodide, the C—S—C thioether bond angle is 101.66 (9)° and electrons are delocalized over the N + = C—N skeleton. The dihedral angle between the aromatic rings attached to the N atoms is 40.60 (9)°. In the crystal, N—H...I hydrogen bonds link the components into [100] chains.

Synthesis and crystal structure of (E)-2-benzyl-1,3-diphenylisothiouronium iodide