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The title compound, [Tl 4 (C 4 H 9 O) 4 ], featuring a (Tl—O) 4  cube, crystallizes with a quarter-mol­ecule (located on a special position of site symmetry..) and a half-mol­ecule (located on a special position of site symmetry 23.) in the asymmetric unit. The Tl—O bond distances range from 2.463 (12) to 2.506 (12) Å. All O—Tl—O bond angles are smaller than 90° whereas the Tl—O—Tl angles are wider than a recta­ngular angle.

Tetra-μ3-tert-butanolato-tetrathallium(I)

Tetra-μ₃-tert-butanolato-tetrathallium(I)